I would say the OHMSS theme (track 6) is Barry at his best. As for The Living Daylights, its his last Bond score and a great one at that, the highlights being Exercise at Gibraltiar, Ice Chase, and Into Vienna. One can also not forget the OO7, used in five different films and a great piece of music. I would also recommend some tracks from Casino Royale, preferablly African Rundown and Blunt Instrument.